Issues $\rightarrow$ Volume 24, Issue 4 (2023)

Hydrogen in Compounds and Alloys with A15 Structure

An. D. Zolotarenko$^{1,2}$, Ol. D. Zolotarenko$^{1,2}$, Z. A. Matysina$^1$, N. A. Shvachko$^{1,3}$, N. Y. Akhanova$^{4,5}$, M. Ualkhanova$^5$, D. V. Schur$^{1,6}$, M. T. Gabdullin$^4$, M. T. Kartel$^2$, Yu. M. Solonin$^1$, Yu. I. Zhirko$^6$, D. V. Ismailov$^{5,7}$, A. D. Zolotarenko$^1$, and I. V. Zagorulko$^8$

$^1$I. M. Frantsevych Institute for Problems of Materials Science of the N.A.S. of Ukraine, Omeljan Pritsak Str., UA-03142 Kyiv, Ukraine
 $^2$O. O. Chuiko Institute of Surface Chemistry of the N.A.S. of Ukraine, 17 General Naumov Str., UA-03164 Kyiv, Ukraine
 $^3$Kyiv National University of Construction and Architecture, 31 Povitroflotskyi Ave., UA-03037 Kyiv, Ukraine
 $^4$Kazakh–British Technical University, 59 Tole bi Str., 050000 Almaty, Kazakhstan
 $^5$Al-Farabi Kazakh National University, 71 Al-Farabi Ave., 050040 Almaty, Kazakhstan
 $^6$Institute of Applied Physics of the N.A.S. of Ukraine, 58 Petropavlivska Str., UA-40000 Sumy, Ukraine
 $^7$NJSC ‘K. I. Satbayev Kazakh National Research Technical University’, 22a Satbaev Str., 050013 Almaty, Kazakhstan
 $^8$G. V. Kurdyumov Institute for Metal Physics of the N.A.S. of Ukraine, 36 Academician Vernadsky Blvd., UA-03142 Kyiv, Ukraine

Received 28.09.2023; final version — 17.11.2023 Download PDF logo PDF

Abstract
In the present work, a theoretical study of atomic ordering in the A3BCx alloy is carried out. The mutual influence of the ordering and solubility of impurity C in the A3B alloy is studied. The dependences of solubility on the composition of the alloy, temperature, degree of long-range order are found and studied. In addition, the criteria for the manifestation of extremity in the concentration and temperature dependences of solubility are obtained. The atomic ordering is studied using the average-energies’ method; the features of the C impurity solubility in the A3B alloy are elucidated using the configuration method. Experiments confirming the results of the theory are currently unknown to authors. However, the available experimental data on determining the temperatures of martensitic transformation (Tm) and superconducting transition (Tc) for the Nb3SnHx alloy allow us to hope and assert a possible agreement between the data of theory and experiment.

Keywords: crystal structure, A15-type structure, alloys, compounds, metal hydrides, hydrogen, phase transformations, order–disorder transitions, solubility.

DOI: https://doi.org/10.15407/ufm.24.04.654

Citation: An. D. Zolotarenko, Ol. D. Zolotarenko, Z. A. Matysina, N. A. Shvachko, N. Y. Akhanova, M. Ualkhanova, D. V. Schur, M. T. Gabdullin, M. T. Kartel, Yu. M. Solonin, Yu. I. Zhirko, D. V. Ismailov, A. D. Zolotarenko, and I. V. Zagorulko, Hydrogen in Compounds and Alloys with A15 Structure, Progress in Physics of Metals, 24, No. 4: 654–685 (2023)

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